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Highly luminescent organic-inorganic hybrid antimony halide scintillators for real-time dynamic and 3D X-ray imaging
This research introduces novel Sb³⁺-based organic-inorganic hybrid halide (OIHH) scintillators, CP1 and CP2, addressing the toxicity and instability issues of lead-based alternatives. CP2, incorporating water molecules, demonstrates superior photoluminescence quantum yield (97.25%) and light yield (32332 photons MeV⁻¹) due to enhanced lattice distortion and reduced non-radiative decay, promoting self-trapped exciton emissions. A flexible scintillator screen made from CP2 crystals achieves high spatial resolution (14 lp mm⁻¹) and excellent environmental stability. The work successfully pioneers the application of Sb³⁺-based OIHHs for real-time dynamic and 3D X-ray imaging, marking a significant advancement in non-toxic, high-performance X-ray detection.
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Photoluminescence Quantum Yield (CP2)
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Light Yield (CP2)
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Spatial Resolution
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Environmental Stability
Deep Analysis & Enterprise Applications
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Details the design, synthesis, and structural analysis of CP1 and CP2 crystals, highlighting the role of water molecules in CP2's enhanced properties.
97.25%
Achieved PLQY for CP2, significantly higher than CP1's 73.38% due to optimized crystal structure.
Enterprise Process Flow
Initial Sb³⁺-OIHH Design (CP1)
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Introduce Water Molecules (CP2)
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Increase Lattice Distortion
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Enhance Self-Trapped Exciton Emissions
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Improve PLQY & Light Yield
Explores the optical properties, light yield, detection limits, and X-ray resistance, demonstrating CP2's superior performance compared to CP1 and BGO.
CP2 vs. CP1 and Commercial BGO Scintillators
| Feature | CP1 | CP2 | BGO (Reference) |
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| Light Yield (photons MeV⁻¹) |
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| PLQY |
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| Lattice Distortion (σ²) |
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| X-ray Detection Limit |
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32332
Photons MeV⁻¹ light yield, outperforming BGO by 3.2 times, indicating high sensitivity.
Covers the fabrication of flexible scintillator screens and their successful application in real-time dynamic and 3D X-ray imaging.
Real-time Dynamic X-ray Imaging of Intricate Objects
The flexible CP2 scintillator film was successfully applied to real-time dynamic X-ray imaging of a curved copper ornament and a flexible circuit. The flexible nature allowed seamless adherence, reducing image distortion from uneven X-ray dose distribution. Resulting in clear, high-resolution internal structures visible at 60 frames per second with no ghosting, demonstrating superior adaptability for non-planar objects.
14 lp mm⁻¹
Spatial resolution achieved by the CP2 flexible scintillator screen, enabling detailed visualization.
3D X-ray Reconstruction of Complex Structures
Utilizing a self-built 360° rotatable platform, the CP2 flexible scintillator film facilitated the collection of X-ray projection photos of a nail at various angles. The subsequent application of the Feldkamp-Davis-Kress (FDK) algorithm enabled a detailed 3D reconstruction of the nail. This pioneering application of Sb³⁺-OIHHs in 3D imaging significantly broadens their potential for advanced material inspection and medical diagnostics.
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